By Pokémon, they all look good. By sprite designs, Yellow had the best.
I always thought that Kinglers sprite was pretty cool.
I remember Yellow being such an improvement over R/B, I know part of it was the fact that we could see the sprites in color now.
As far as R/B is concerned, I think pretty much from Staryu until Mewtwo, with a few exceptions (Articuno and Moltres for example), pretty much retain their same style today.
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I think that dratini and dragonair look pretty good in yellow. They are the right colors!
I have claimed Electabuzz!
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Nidoking and Nidoqueen have good sprites, look identical to their art.
Now, I should beat Blue for the full pokedex!
So far, Red, Silver, Ruby, Sapphire, and Diamond are complete.
Games to finish: Blue, Emerald, Firered, Soulsilver and White 2 to go... (At least I have summer to run through these games! )
I loved Squirtle's sprite. Gengar's was cool as well
Pokemon Black 2 Team:
Beedrill looked badass in yellow.
For sprites I liked, Staryu, Jolteon, Zapados, Lapras, Jigglypuff & (of course) Pikachu.
Arcanine looked awesome in the Yellow Version
Lucario: Master of Aura...... and Chocolate!
I love Jolteon in Green! He looks so happy and talkative. (Don't ask me how a pokemon can look talkative, but Jolteon does.)
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I like Dragonite's sprites in Red/Blue and Yellow. They actually looked "tough" and aggressive which when I think of a Dragon with strength like Dragonite has I want it to look like that. The later gen's after it made Dragonite look more like a gentle teddy bear.
I like yellow's sprite for Geodude. It's nicely shaded, it's in a cool pose, and it resembles it's anime counterpart.
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I quite like all of Gravelers Gen 1 designs.
Its too bad Golems gen 1 sprites are pretty bad..